Because Smeargle is a special type of pokemon i made him learn these moves:
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False Swipes, What this does is lower the pokemons HP to 1 so that it can be caught a whole lot easier.
Spore, What this does it put the opponent to sleep with 100% chance so that it will be easier to catch.
Mean Look, This move makes it so that no one can escape which is great or Legendary pokemon that try to run away such as Mesprit and Cresselia.
Swords Dance, This move greatly increases your attack to make battles alot easier